Search Advanced
2025 Volume 34 Issue 5
Article Contents
Previous Article Next Article

Yuanjie Yang(杨元杰), Shengran Lin(林盛然), Jiaxin Zhao(赵嘉昕), Changfeng Weng(翁长风), Liren Lou(楼立人), Wei Zhu(祝巍)†, and Guanzhong Wang(王冠中)‡. 2025: Ultrahigh concentration of NV- centers embedded in the CVD epi-diamond layer near the interface with an HPHT diamond substrate, Chinese Physics B, 34(5): 056102. doi: 10.1088/1674-1056/adc7f5
Citation: Yuanjie Yang(杨元杰), Shengran Lin(林盛然), Jiaxin Zhao(赵嘉昕), Changfeng Weng(翁长风), Liren Lou(楼立人), Wei Zhu(祝巍)†, and Guanzhong Wang(王冠中)‡. 2025: Ultrahigh concentration of NV- centers embedded in the CVD epi-diamond layer near the interface with an HPHT diamond substrate, Chinese Physics B, 34(5): 056102. doi: 10.1088/1674-1056/adc7f5
shu

Ultrahigh concentration of NV- centers embedded in the CVD epi-diamond layer near the interface with an HPHT diamond substrate

  • Department of Physics, University of Science and Technology of China, Hefei 230026, China

  • Received Date: 19/02/2025
    Accepted Date: 24/03/2025
  • Fund Project:

    Project supported by the National Natural Science Foundation of China (Grant Nos. 11374280 and 50772110).

  • PACS: 61.72.J-; 81.05.ug; 68.35.Ct; 71.55.-i

  • The negatively charged nitrogen vacancy (NV$^-$) center ensemble in as-grown chemical vapor deposition (CVD) diamond is a promising candidate for quantum sensing due to its long coherence time and excellent optical properties. However, achieving a high concentration of NV$^-$ centers in as-grown CVD diamond remains a critical challenge, which constrains the performance of NV$^-$ based sensors. In this study, we observe that NV$^-$ center formation efficiency is significantly enhanced during the initial growth phase, with a coherence time $T^*_2$ of 1.1 μs. These findings demonstrate that high-concentration NV$^-$ centers can be achieved in as-grown diamonds, greatly enhancing their utility in high-performance magnetometers and quantum sensing.
  • 加载中
  • Takeuchi M, Yasuoka M, Ishii M, Ohtani N and Shikata S 2023 Diam. Relat. Mater. 140 110510

    Google Scholar Pub Med

    Zou D, Shen S, Li L, Wang Q, Liang K, Chen L, Wu G and Shen W 2024 Phys. B 676 415614

    Google Scholar Pub Med

    Bai R, Zhu X, Yang F, Gao T, Wang Z, Yu L, Wang J, Zhou L and Du G 2022 Chin. Phys. B 31 074203

    Google Scholar Pub Med

    Wang J, Feng F, Zhang J, Chen J, Zheng Z, Guo L, Zhang W, Song X, Guo G, Fan L, Zou C, Lou L, Zhu W and Wang G 2015 Phys. Rev. B 91 155404

    Google Scholar Pub Med

    Xu K, Xie T, Li Z, Xu X, Wang M, Ye X, Kong F, Geng J, Duan C, Shi F and Du J 2017 Phys. Rev. Lett. 118 130504

    Google Scholar Pub Med

    Masuyama Y, Suzuki K, Hekizono A, Iwanami M, Hatano M, Iwasaki T and Ohshima T 2021 Sensors 21 977

    Google Scholar Pub Med

    Budakian R, Finkler A, Eichler A, Poggio M, Degen C L, Tabatabaei S, Lee I, Hammel P C, Eugene S P, Taminiau T H, Walsworth R L, London P, Bleszynski Jayich A, Ajoy A, Pillai A, Wrachtrup J, Jelezko F, Bae Y, Heinrich A J, Ast C R, Bertet P, Cappellaro P, Bonato C, Altmann Y and Gauger E 2024 Nanotechnology 35 412001

    Google Scholar Pub Med

    Atatüre M, Englund D, Vamivakas N, Lee S Y and Wrachtrup J 2018 Nat. Rev. Mater. 3 38

    Google Scholar Pub Med

    Delle Donne C, Iuliano M, Van Der Vecht B, Ferreira G M, Jirovská H, Van Der Steenhoven T J W, Dahlberg A, Skrzypczyk M, Fioretto D, Teller M, Filippov P, Montblanch A R P, Fischer J, Van Ommen H B, Demetriou N, Leichtle D, Music L, Ollivier H, Te Raa I, Kozlowski W, Taminiau T H, Pawełczak P, Northup T E, Hanson R and Wehner S 2025 Nature 639 321

    Google Scholar Pub Med

    Shandilya P K, Flagan S, Carvalho N C, Zohari E, Kavatamane V K, Losby J E and Barclay P E 2022 J. Light. Technol. 40 7538

    Google Scholar Pub Med

    Basu T, Patra A, Murali M, Saini M, Banerjee A and Som 2025 ACS Omega 10 2372

    Google Scholar Pub Med

    Liu X, Cui J, Sun F, Song X, Feng F, Wang J, Zhu W, Lou L and Wang G 2013 Appl. Phys. Lett. 103 143105

    Google Scholar Pub Med

    Hei L F, Zhao Y, Wei J J, Liu J L, Li C M, Tang W Z and Lu F X 2016 Diam. Relat. Mater. 69 33

    Google Scholar Pub Med

    Samlenski R, Haug C, Brenn R, Wild C, Locher R and Koidl P 1995 Appl. Phys. Lett. 67 2798

    Google Scholar Pub Med

    Feng F, Wang J, Zhang W, Zhang J, Lou L, Zhu W and Wang G 2016 Appl. Phys. A 122 944

    Google Scholar Pub Med

    Yokota Y, Kawarada H and Hiraki A 1990 Jpn. J. Appl. Phys. 29 L2232

    Google Scholar Pub Med

    Romach Y, Müller C, Unden T, Rogers L J, Isoda T, Itoh K M, Markham M, Stacey A, Meijer J, Pezzagna S, Naydenov B, McGuinness L P, Bar-Gill N and Jelezko F 2015 Phys. Rev. Lett. 114 017601

    Google Scholar Pub Med

    Hounsome L S, Jones R, Martineau P M, Fisher D, Shaw M J, Briddon P R and Ö berg S 2006 Phys. Rev. B 73 125203

    Google Scholar Pub Med

    Ohno K, Joseph Heremans F, Bassett L C, Myers B A, Toyli D M, Bleszynski Jayich A C, Palmstrøm C J and Awschalom D D 2012 Appl. Phys. Lett. 101 082413

    Google Scholar Pub Med

    Tallaire A, Achard J, Silva F, Sussmann R S, Gicquel A and Rzepka E 2004 Phys. Status Solidi A 201 2419

    Google Scholar Pub Med

    Woods G S, Van Wyk J A and Collins A T 1990 Philos. Mag. B 62 589

    Google Scholar Pub Med

    Liu J L, Zheng Y T, Lin L Z, Zhao Y, Chen L X, Wei J J, Wang J J, Guo J C, Feng Z H and Li C M 2018 J. Mater. Sci. 53 13030

    Google Scholar Pub Med

    Tallaire A, Mayer L, Brinza O, Pinault-Thaury M A, Debuisschert T and Achard J 2017 Appl. Phys. Lett. 111 143101

    Google Scholar Pub Med

    Anon

    Google Scholar Pub Med

    Martineau P M, Lawson S C, Taylor A J, Quinn S J, Evans D J F and Crowder M J 2004 Gems Gemol. 40 2

    Google Scholar Pub Med

    Edmonds A M, D’Haenens-Johansson U F S, Cruddace R J, NewtonM E, Fu K M C, Santori C, Beausoleil R G, Twitchen D J and Markham M L 2012 Phys. Rev. B 86 035201

    Google Scholar Pub Med

    Bou P, Vandenbulcke L, Herbin R and Hillion F 1992 J. Mater. Res. 7 2151

    Google Scholar Pub Med

    Dréau A, Lesik M, Rondin L, Spinicelli P, Arcizet O, Roch J F and Jacques V 2011 Phys. Rev. B 84 195204

    Google Scholar Pub Med

    Hu X, Liu G Q, Xu Z C and Pan X Y 2012 Chin. Phys. Lett. 29 024210

    Google Scholar Pub Med

    Dutt M V G, Childress L, Jiang L, Togan E, Maze J, Jelezko F, Zibrov A S, Hemmer P R and Lukin M D 2007 Science 316 1312

    Google Scholar Pub Med

    Ding S, Zhang J, Su K, Ren Z, Chen J, Yang Z, Zhang J and Hao Y 2024 Sci. China Mater. 67 2329

    Google Scholar Pub Med

    Acosta V M, Bauch E, Ledbetter M P, Santori C, Fu K M C, Barclay P E, Beausoleil R G, Linget H, Roch J F, Treussart F, Chemerisov S, Gawlik W and Budker D 2009 Phys. Rev. B 80 115202

    Google Scholar Pub Med

    Kleinsasser E E, Stanfield M M, Banks J K Q, Zhu Z, Li W D, Acosta V M, Watanabe H, Itoh K M and Fu K M C 2016 Appl. Phys. Lett. 108 202401

    Google Scholar Pub Med

    Maertz B J, Wijnheijmer A P, Fuchs G D, Nowakowski M E and Awschalom D D 2010 Appl. Phys. Lett. 96 092504

    Google Scholar Pub Med

    Le Sage D, Pham L M, Bar-Gill N, Belthangady C, LukinMD, Yacoby A and Walsworth R L 2012 Phys. Rev. B 85 121202

    Google Scholar Pub Med

  • 加载中
通讯作者: 陈斌, bchen63@163.com
  • 1. 

    沈阳化工大学材料科学与工程学院 沈阳 110142

  1. 本站搜索
  2. 百度学术搜索
  3. 万方数据库搜索
  4. CNKI搜索
Export Citation
PDF
XML

Article Metrics

Article views(174) PDF downloads(0) Cited by(0)

Access History

Ultrahigh concentration of NV- centers embedded in the CVD epi-diamond layer near the interface with an HPHT diamond substrate

  • Received Date: 19/02/2025
  • Accepted Date: 24/03/2025
Fund Project: 

Abstract: The negatively charged nitrogen vacancy (NV$^-$) center ensemble in as-grown chemical vapor deposition (CVD) diamond is a promising candidate for quantum sensing due to its long coherence time and excellent optical properties. However, achieving a high concentration of NV$^-$ centers in as-grown CVD diamond remains a critical challenge, which constrains the performance of NV$^-$ based sensors. In this study, we observe that NV$^-$ center formation efficiency is significantly enhanced during the initial growth phase, with a coherence time $T^*_2$ of 1.1 μs. These findings demonstrate that high-concentration NV$^-$ centers can be achieved in as-grown diamonds, greatly enhancing their utility in high-performance magnetometers and quantum sensing.

    HTML

Reference (35)

Catalog

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return